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Trzeciecki, M., Dähn, A., Hübner, W.

Symmetry analysis of second-harmonic generation at surfaces of antiferromagnets
Physical Review B 60, (2),pp 1144-1160 (1999)
Using group theory we classify the nonlinear magneto-optical response at low-index surfaces of fee antiferromagnets, such as NiO. Structures consisting of one atomic layer are discussed in detail. We find that optical second-harmonic generation is sensitive to surface antiferromagnetism in many cases. We discuss the influence of a second type of magnetic atoms, and also of a possible oxygen sublattice distortion on the output signal. Finally, our symmetry analysis yields the possibility of antiferromagnetic surface domain imaging even in the presence of magnetic unit-cell doubling.

ki-1999-s10